@article{oai:oist.repo.nii.ac.jp:00001708, author = {Liu, Zonghao and Qiu, Longbin and Ono, Luis K. and He, Sisi and Hu, Zhanhao and Jiang, Maowei and Tong, Guoqing and Wu, Zhifang and Jiang, Yan and Son, Dae-Yong and Dang, Yangyang and Kazaoui, Said and Qi, Yabing}, issue = {8}, journal = {Nature Energy}, month = {Jul}, note = {The upscaling of perovskite solar cells to module scale and long-term stability have been recognized as the most important challenges for the commercialization of this emerging photovoltaic technology. In a perovskite solar module, each interface within the device contributes to the efficiency and stability of the module. Here, we employed a holistic interface stabilization strategy by modifying all the relevant layers and interfaces, namely the perovskite layer, charge transporting layers and device encapsulation, to improve the efficiency and stability of perovskite solar modules. The treatments were selected for their compatibility with low-temperature scalable processing and the module scribing steps. Our unencapsulated perovskite solar modules achieved a reverse-scan efficiency of 16.6% for a designated area of 22.4 cm². The encapsulated perovskite solar modules, which show efficiencies similar to the unencapsulated one, retained approximately 86% of the initial performance after continuous operation for 2,000 h under AM1.5G light illumination, which translates into a T₉₀ lifetime (the time over which the device efficiency reduces to 90% of its initial value) of 1,570 h and an estimated T80 lifetime (the time over which the device efficiency reduces to 80% of its initial value) of 2,680 h.}, pages = {596--604}, title = {A holistic approach to interface stabilization for efficient perovskite solar modules with over 2,000-hour operational stability}, volume = {5}, year = {2020} }