{"created":"2023-06-26T11:01:13.767895+00:00","id":1891,"links":{},"metadata":{"_buckets":{"deposit":"66778197-3f12-4957-9c0f-a9310dedbf36"},"_deposit":{"created_by":30,"id":"1891","owners":[30],"pid":{"revision_id":0,"type":"depid","value":"1891"},"status":"published"},"_oai":{"id":"oai:oist.repo.nii.ac.jp:00001891","sets":["6:177"]},"author_link":["12143","12148","12150","12151","12145","12152","12142","12147","12141","12146","12144","12153","12149"],"item_10001_biblio_info_7":{"attribute_name":"Bibliographic Information","attribute_value_mlt":[{"bibliographicIssueDates":{"bibliographicIssueDate":"2020-11-18","bibliographicIssueDateType":"Issued"},"bibliographicIssueNumber":"1","bibliographicPageStart":"5892","bibliographicVolumeNumber":"11","bibliographic_titles":[{},{"bibliographic_title":"Nature Communications","bibliographic_titleLang":"en"}]}]},"item_10001_creator_3":{"attribute_name":"Author","attribute_type":"creator","attribute_value_mlt":[{"creatorNames":[{"creatorName":"Zhou, Yazhou"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Tao, Xiafang"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Chen, Guangbo"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Lu, Ruihu"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Wang, Ding"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Chen, Ming-Xi"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Jin, Enquan"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Yang, Juan"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Liang, Hai-Wei"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Zhao, Yan"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Feng, Xinliang"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Narita, Akimitsu"}],"nameIdentifiers":[{}]},{"creatorNames":[{"creatorName":"Müllen, Klaus"}],"nameIdentifiers":[{}]}]},"item_10001_description_5":{"attribute_name":"Abstract","attribute_value_mlt":[{"subitem_description":"Metal single-atom catalysts (M-SACs) have emerged as an attractive concept for promoting heterogeneous reactions, but the synthesis of high-loading M-SACs remains a challenge. Here, we report a multilayer stabilization strategy for constructing M-SACs in nitrogen-, sulfur- and fluorine-co-doped graphitized carbons (M=Fe, Co, Ru, Ir and Pt). Metal precursors are embedded into perfluorotetradecanoic acid multilayers and are further coated with polypyrrole prior to pyrolysis. Aggregation of the metals is thus efficiently inhibited to achieve M-SACs with a high metal loading (similar to 16wt%). Fe-SAC serves as an efficient oxygen reduction catalyst with half-wave potentials of 0.91 and 0.82V (versus reversible hydrogen electrode) in alkaline and acid solutions, respectively. Moreover, as an air electrode in zinc-air batteries, Fe-SAC demonstrates a large peak power density of 247.7mWcm⁻² and superior long-term stability(.) Our versatile method paves an effective way to develop high-loading M-SACs for various applications.","subitem_description_type":"Other"}]},"item_10001_publisher_8":{"attribute_name":"Publisher","attribute_value_mlt":[{"subitem_publisher":"Nature Research"}]},"item_10001_relation_13":{"attribute_name":"PubMedNo.","attribute_value_mlt":[{"subitem_relation_type":"isIdenticalTo","subitem_relation_type_id":{"subitem_relation_type_id_text":"info:pmid/33208746","subitem_relation_type_select":"PMID"}}]},"item_10001_relation_14":{"attribute_name":"DOI","attribute_value_mlt":[{"subitem_relation_type":"isIdenticalTo","subitem_relation_type_id":{"subitem_relation_type_id_text":"info:doi/10.1038/s41467-020-19599-8","subitem_relation_type_select":"DOI"}}]},"item_10001_relation_17":{"attribute_name":"Related site","attribute_value_mlt":[{"subitem_relation_type_id":{"subitem_relation_type_id_text":"https://www.nature.com/articles/s41467-020-19599-8","subitem_relation_type_select":"URI"}}]},"item_10001_rights_15":{"attribute_name":"Rights","attribute_value_mlt":[{"subitem_rights":"© 2020 The Author(s)."}]},"item_10001_source_id_9":{"attribute_name":"ISSN","attribute_value_mlt":[{"subitem_source_identifier":"2041-1723","subitem_source_identifier_type":"ISSN"}]},"item_10001_version_type_20":{"attribute_name":"Author's flag","attribute_value_mlt":[{"subitem_version_resource":"http://purl.org/coar/version/c_970fb48d4fbd8a85","subitem_version_type":"VoR"}]},"item_files":{"attribute_name":"ファイル情報","attribute_type":"file","attribute_value_mlt":[{"accessrole":"open_date","date":[{"dateType":"Available","dateValue":"2021-01-19"}],"displaytype":"detail","filename":"Zhou-2020-Multilayer stabilization for fabrica.pdf","filesize":[{"value":"2.9 MB"}],"format":"application/pdf","license_note":"Creative Commons Attribution 4.0 International(https://creativecommons.org/licenses/by/4.0/)","licensetype":"license_note","mimetype":"application/pdf","url":{"label":"Zhou-2020-Multilayer stabilization for fabrica","url":"https://oist.repo.nii.ac.jp/record/1891/files/Zhou-2020-Multilayer stabilization for fabrica.pdf"},"version_id":"0577cd36-4ef2-49cc-91a9-4fbe5f778160"}]},"item_language":{"attribute_name":"言語","attribute_value_mlt":[{"subitem_language":"eng"}]},"item_resource_type":{"attribute_name":"資源タイプ","attribute_value_mlt":[{"resourcetype":"journal article","resourceuri":"http://purl.org/coar/resource_type/c_6501"}]},"item_title":"Multilayer stabilization for fabricating high-loading single-atom catalysts","item_titles":{"attribute_name":"タイトル","attribute_value_mlt":[{"subitem_title":"Multilayer stabilization for fabricating high-loading single-atom catalysts","subitem_title_language":"en"}]},"item_type_id":"10001","owner":"30","path":["177"],"pubdate":{"attribute_name":"公開日","attribute_value":"2021-01-19"},"publish_date":"2021-01-19","publish_status":"0","recid":"1891","relation_version_is_last":true,"title":["Multilayer stabilization for fabricating high-loading single-atom catalysts"],"weko_creator_id":"30","weko_shared_id":30},"updated":"2023-06-26T11:41:00.389124+00:00"}