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Scalable Fabrication of >90 cm2 Perovskite Solar Modules with >1000 h Operational Stability Based on the Intermediate Phase Strategy
https://oist.repo.nii.ac.jp/records/1976
https://oist.repo.nii.ac.jp/records/1976506b4f30-45e6-442f-a92d-e7d5259cd927
| 名前 / ファイル | ライセンス | アクション |
|---|---|---|
MS (4.5 MB)
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| Item type | 学術雑誌論文 / Journal Article(1) | |||||
|---|---|---|---|---|---|---|
| 公開日 | 2021-03-11 | |||||
| タイトル | ||||||
| タイトル | Scalable Fabrication of >90 cm2 Perovskite Solar Modules with >1000 h Operational Stability Based on the Intermediate Phase Strategy | |||||
| 言語 | en | |||||
| 言語 | ||||||
| 言語 | eng | |||||
| キーワード | ||||||
| 言語 | en | |||||
| 主題Scheme | Other | |||||
| 主題 | intermediate phase | |||||
| キーワード | ||||||
| 言語 | en | |||||
| 主題Scheme | Other | |||||
| 主題 | operational stability | |||||
| キーワード | ||||||
| 言語 | en | |||||
| 主題Scheme | Other | |||||
| 主題 | perovskite solar cells | |||||
| キーワード | ||||||
| 言語 | en | |||||
| 主題Scheme | Other | |||||
| 主題 | scalability | |||||
| キーワード | ||||||
| 言語 | en | |||||
| 主題Scheme | Other | |||||
| 主題 | solar modules | |||||
| 資源タイプ | ||||||
| 資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
| 資源タイプ | journal article | |||||
| 著者（英） |
Tong, Guoqing
× Tong, Guoqing× Son, Dae‐Yong× Ono, Luis K.× Liu, Yuqiang× Hu, Yanqiang× Zhang, Hui× Jamshaid, Afshan× Qiu, Longbin× Liu, Zonghao× Qi, Yabing |
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| 書誌情報 |
en : Advanced Energy Materials 巻 11, 号 10, p. 2003712, 発行日 2021-01-25 |
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| 抄録 | ||||||
| 内容記述タイプ | Other | |||||
| 内容記述 | In addition to high efficiencies, upscaling and long‐term operational stability are key pre‐requisites for moving perovskite solar cells toward commercial applications. In this work, a strategy to fabricate large‐area uniform and dense perovskite films with a thickness over one‐micrometer via a two‐step coating process by introducing NH4Cl as an additive in the PbI2 precursor solution is developed. Incorporation of NH4Cl induces the formation of the intermediate phases of x[NH4+]·[PbI2Clx]x− and HPbI3−xClx, which can effectively retard the crystallization rate of perovskite leading to uniform and compact full‐coverage perovskite layers across large areas with high crystallinity, large grain sizes, and small surface roughness. The 5 × 5 and 10 × 10 cm2 perovskite solar modules (PSMs) based on this method achieve a power conversion efficiency (PCE) of 14.55% and 10.25%, respectively. These PSMs also exhibit good operational stability with a T80 lifetime (the time during which the solar module PCE drops to 80% of its initial value) under continuous light illumination exceeding 1600 h (5 × 5 cm2) and 1100 h (10 × 10 cm2), respectively. | |||||
| 出版者 | ||||||
| 出版者 | Wiley | |||||
| ISSN | ||||||
| 収録物識別子タイプ | ISSN | |||||
| 収録物識別子 | 1614-6832 | |||||
| ISSN | ||||||
| 収録物識別子タイプ | ISSN | |||||
| 収録物識別子 | 1614-6840 | |||||
| DOI | ||||||
| 関連タイプ | isVersionOf | |||||
| 識別子タイプ | DOI | |||||
| 関連識別子 | info:doi/10.1002/aenm.202003712 | |||||
| 権利 | ||||||
| 権利情報 | This is the peer reviewed version of the following article: Guoqing Tong, Dae‐Yong Son, Luis K. Ono, Yuqiang Liu, Yanqiang Hu, Hui Zhang, Afshan Jamshaid, Longbin Qiu, Zonghao Liu, Yabing Qi, Scalable Fabrication of >90 cm2 Perovskite Solar Modules with >1000 h Operational Stability Based on the Intermediate Phase Strategy, Advanced Energy Materials, 2021: 2003712.,which has been published in final form at https://doi.org/10.1002/aenm.202003712. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions. | |||||
| 関連サイト | ||||||
| 識別子タイプ | URI | |||||
| 関連識別子 | https://onlinelibrary.wiley.com/doi/10.1002/aenm.202003712 | |||||
| 著者版フラグ | ||||||
| 出版タイプ | AM | |||||
| 出版タイプResource | http://purl.org/coar/version/c_ab4af688f83e57aa | |||||
