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Improved SnO2 Electron Transport Layers Solution-Deposited at Near Room Temperature for Rigid or Flexible Perovskite Solar Cells with High Efficiencies
https://oist.repo.nii.ac.jp/records/1323
https://oist.repo.nii.ac.jp/records/1323d5f695ee-a5c7-41d4-b075-629ffaeffa30
名前 / ファイル | ライセンス | アクション |
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Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2020-03-24 | |||||
タイトル | ||||||
言語 | en | |||||
タイトル | Improved SnO2 Electron Transport Layers Solution-Deposited at Near Room Temperature for Rigid or Flexible Perovskite Solar Cells with High Efficiencies | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
資源タイプ | journal article | |||||
著者(英) |
Dong, Qingshun
× Dong, Qingshun× Li, Jiangwei× Shi, Yantao× Chen, Min× Ono, Luis K.× Zhou, Ke× Zhang, Chunyang× Qi, Yabing× Zhou, Yuanyuan× Padture, Nitin P.× Wang, Liduo |
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書誌情報 |
en : Advanced Energy Materials 巻 9, 号 26, p. 1900834, 発行日 2019-05-28 |
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抄録 | ||||||
内容記述タイプ | Other | |||||
内容記述 | Electron transport layer (ETL) is a functional layer of great significance for boosting the power conversion efficiency (PCE) of perovskite solar cells (PSCs). To date, it is still a challenge to simultaneously reduce the surface defects and improve the crystallinity in ETLs during their low-temperature processing. Here, a novel strategy for the mediation of in situ regrowth of SnO2 nanocrystal ETLs is reported: introduction of controlled trace amounts of surface absorbed water on the fluorinated tin oxide (FTO) or indium-tin oxide (ITO) surfaces of the substrates using ultraviolet ozone (UVO) pretreatment. The optimum amount of adsorbed water plays a key role in balancing the hydrolysis-condensation reactions during the structural evolution of SnO2 thin films. This new approach results in a full-coverage SnO2 ETL with a desirable morphology and crystallinity for superior optical and electrical properties, as compared to the control SnO2 ETL without the UVO pretreatment. Finally, the rigid and flexible PSC devices based on the new SnO2 ETLs yield high PCEs of up to 20.5% and 17.5%, respectively. | |||||
出版者 | ||||||
出版者 | John Wiley & Sons, Inc. | |||||
ISSN | ||||||
収録物識別子タイプ | ISSN | |||||
収録物識別子 | 1614-6832 | |||||
ISSN | ||||||
収録物識別子タイプ | ISSN | |||||
収録物識別子 | 1614-6840 | |||||
DOI | ||||||
関連タイプ | isVersionOf | |||||
識別子タイプ | DOI | |||||
関連識別子 | info:doi/10.1002/aenm.201900834 | |||||
権利 | ||||||
権利情報 | © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim | |||||
権利 | ||||||
権利情報 | This is the accepted version of the following article: Dong, Q., Li, J., Shi, Y., Chen, M., Ono, L. K., Zhou, K., Zhang, C., Qi, Y., Zhou, Y., Padture, N. P., Wang, L., Improved SnO2 Electron Transport Layers Solution‐Deposited at Near Room Temperature for Rigid or Flexible Perovskite Solar Cells with High Efficiencies. Adv. Energy Mater. 2019, 9, 1900834, which has been published in final form at https://doi.org/10.1002/aenm.201900834. This article may be used for non-commercial purposes in accordance with the Wiley Self-Archiving Policy [https://authorservices.wiley.com/authorresources/Journal-Authors/licensing/self-archiving.html]. | |||||
関連サイト | ||||||
識別子タイプ | DOI | |||||
関連識別子 | https://doi.org/10.1002/aenm.201900834 | |||||
著者版フラグ | ||||||
出版タイプ | AM | |||||
出版タイプResource | http://purl.org/coar/version/c_ab4af688f83e57aa |